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Author Topic: The Science of Aerosols  (Read 121649 times)

kassy

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Re: The Science of Aerosols
« Reply #300 on: March 05, 2023, 03:46:30 PM »
Quote from: Human Habitat Index link=topic=1384.msg361067#msg361067
If Australia used more coal would it cool the continent in the short and long term ?
[/quote

No. There should be a slight change but it would not offset the global changes in temperature (big ocean next to you).
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jai mitchell

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Re: The Science of Aerosols
« Reply #301 on: June 07, 2023, 06:00:38 PM »
Cross Posted

Nair et. al.

https://www.nature.com/articles/s41612-023-00367-6

Aerosol demasking enhances climate warming over South Asia

Quote
Concurrent measurements over the northern Indian Ocean unveiled a ~7% increase in the earth’s surface-reaching solar radiation (surface brightening). Aerosol-induced atmospheric solar heating decreased by ~0.4 K d−1. Our results reveal that under clear sky conditions, anthropogenic emissions over South Asia lead to nearly 1.4 W m−2 heating at the top of the atmosphere during the period March–May. A complete phase-out of today’s fossil fuel combustion to zero-emission renewables would result in rapid aerosol demasking, while the GHGs linger on.

The amount of aerosol forcing is much higher than modeled.  The impacts of this forcing on global atmosphere circulation is much more than modeled.
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morganism

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Re: The Science of Aerosols
« Reply #302 on: August 22, 2023, 11:29:41 PM »
New technology developed for time-resolved measurement of hydroxyl radicals

Researchers led by Prof. Zhang Weijun from the Hefei Institutes of Physical Science of the Chinese Academy of Sciences have proposed a feasible approach for the rapid detection of hydroxyl radicals.

Based on this technology, a new device called Frequency-modulated Faraday Rotation (FM-FRS) spectrometer has been developed, which can detect OH radicals with high precision. The study was published in Optics Express.

Hydroxyl (OH) radicals are important active oxidants in the atmosphere and are important reaction chain initiators in the oxidation of most compounds. In order to study their reaction processes and mechanisms in detail, they must be measured directly in "real time," i.e., to study them on the time scale of their actual existence. Therefore, detection techniques must be able to respond to rapid changes in the concentration and lifetime of OH radicals.

To address this problem, the researchers developed the FM-FRS spectrometer for highly sensitive and rapid measurement of OH radicals, which was characterized by wide measurement bandwidth, high sensitivity, and good selectivity, and is particularly suitable for kinetic studies of short-lived intermediate radicals.

"We used a special laser beam that is modulated at a very high frequency, up to 150 million times per second," said Cheng Feihu, a member of the team.
Concentration-time profile of OH radical obtained after averaging three pulses at a 200 μs sampling interval.

The researchers used the spectroscopic technique to measure the time-resolved spectral signal of the OH radical near 2.8 μm. The detection limit for OH reached 6.8×108 molecules/cm3 (1σ, 0.2 ms) after three pulse averaging, and decreased to 8.0×107 molecules/cm3 after 100 event integrations, which was in general agreement with the trend of the system performance in the white noise limit.

This work provides a new and alternative tool for studying radical dynamics, not only for OH radicals, but also for other paramagnetic transient molecules.

More information: Feihu Cheng et al, High band-width mid-infrared frequency-modulated Faraday rotation spectrometer for time resolved measurement of the OH radical, Optics Express (2023). DOI: 10.1364/OE.493270

https://phys.org/news/2023-08-technology-time-resolved-hydroxyl-radicals.html

vox_mundi

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Re: The Science of Aerosols
« Reply #303 on: April 12, 2024, 02:13:39 PM »
Study Presents Evidence That Recent Reductions In Aerosol Emissions Create an Additional Warming Effect
https://phys.org/news/2024-04-evidence-reductions-aerosol-emissions-additional.html



Recent reductions in emissions of tiny particles, the major cause of air pollution globally, have led to more heat in the Earth's climate system. This is shown in a new international study led by CICERO and published in Communications Earth & Environment.

Satellite measurements clearly show that more heat is entering the Earth's atmosphere from the sun compared to the amount of terrestrial energy escaping to space. This so-called Earth energy imbalance leads to accumulation of heat and warming of the Earth's surface.

In the study, the researchers performed simulations using the latest generation global climate models and compared their results to satellite measurements of the Earth's energy imbalance trend over the 2001–2019 period.

The authors found that the recent reductions in man-made particle emissions needed to be accounted for in order for the models to reasonably match the satellite measurements (see figure above; black vs. orange line). When the authors assumed that the particle emissions did not change over the time period (green line), the simulated heating of the Earth was considerably reduced.

... Hodnebrog says, "Continued reductions of particle emissions may lead to an accelerated surface temperature warming already in this decade."

Øivind Hodnebrog et al, Recent reductions in aerosol emissions have increased Earth's energy imbalance, Communications Earth & Environment[/u] (2024)
https://www.nature.com/articles/s43247-024-01324-8
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kiwichick16

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Re: The Science of Aerosols
« Reply #304 on: April 13, 2024, 05:46:48 AM »
correct me if i'm wrong , but i think Hansen referred to it as " our Faustian bargain " in his book "Storms of my Grandchildren "

kassy

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Re: The Science of Aerosols
« Reply #305 on: April 25, 2024, 11:26:19 AM »
Air Pollution Has Masked Climate Change’s Influence on U.S. Rainfall

As greenhouse gas emissions raise the temperature of the atmosphere, scientists expect global rainfall to increase, but making regional precipitation predictions is challenging. And it’s at the regional level that these predictions are most important for many. Farmers and water managers need to make plans and adjust to climate change.

“Especially for rainfall, what’s happening locally is really important,” said Mark Risser, a climate scientist at Lawrence Berkeley National Laboratory. Risser is an author of a recent study published in Nature Communications that aimed to clarify rainfall trends in the United States by incorporating data about aerosol air pollution. Aerosols are small floating particles that have a drying effect on global climate. Some sources of aerosols are natural, such as sea spray and volatile organic compounds released by plants. There are also anthropogenic sources, such as emissions from the burning of fossil fuels.

The research suggested that climate-change-driven rainfall increases in the United States have been offset by historically high levels of aerosol pollution. But because aerosol levels have fallen in recent decades, thanks to passage of the Clean Air Act in 1970, we are beginning to see more heavy rainfall. Factoring this pollution into climate models can make regional trends clearer, Risser said.

“The implication is that aerosols have been disguising the effects of greenhouse gases on rainfall,” he said. “We unmasked changes happening behind the scenes.”

Small Particles, Big Influence
Precipitation levels vary highly from year to year. It’s extremely challenging to separate the slow changes wrought by global warming from these yearly trends, said Jesse Norris, who studies precipitation at the University of California, Los Angeles Center for Climate Science. Norris was not involved with the study.

As concentrations of greenhouse gases in the atmosphere increase, Earth gets hotter. Warmer air can hold more water vapor, and warmer oceans are more prone to evaporation. This should result in more rain, said Risser. For every degree Celsius the average temperature rises, there should be a 7% increase in global average precipitation, but this trend doesn’t always appear in regional precipitation data. “When zooming in on the U.S., this wasn’t showing up in the data,” Risser said.

Risser said the complex effects of aerosols have made it more challenging to clearly see how climate change is influencing precipitation. The aerosols examined in the study offset the effect of greenhouse gases by reflecting solar energy back out into space and cooling the planet. But these aerosols can also have localized impacts on precipitation. That’s because aerosols can influence what kinds of clouds form and how water droplets form within those clouds, said Risser. So depending on the season and local conditions, aerosols can also drive the formation of severe storms, as was in the case of Hurricane Harvey.

...

After 1970, SO2 aerosol emissions in the United States fell gradually but in the past 20 years have gone back to preindustrial levels, said Risser. Norris said it has taken some time for the climate impacts of this to emerge in data because aerosols can persist in the atmosphere for years. “The impact of those aerosols not being emitted is becoming clear now,” Norris said.

Risser and his team used 120-year rainfall records to study both extreme and average rainfall trends. They separated these trends by regions and by seasons and combined these data with emissions estimates of both greenhouse gases and SO2, one of the best-studied aerosols.

After accounting for SO2 aerosol and greenhouse gas emissions, Risser said, global rainfall trends become more evident. Increasing greenhouse gas levels cause increased average and extreme rainfall across all seasons in the United States.

The study also looked at seasonal emissions and precipitation trends, dividing the country into 25-kilometer boxes. In winter and spring, the study found, higher local aerosol emissions lead to drier conditions. In summer and fall, the opposite is true. These seasonal trends are clearest in the northeastern and southeastern United States and in the Great Plains. For the western United States, Risser said, the study is less conclusive. “There’s a lot more year-to-year variation in rainfall in the western U.S., which makes it harder to attribute changes to greenhouse gases or aerosols,” he said.

...

https://eos.org/articles/air-pollution-has-masked-climate-changes-influence-on-u-s-rainfall
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morganism

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Re: The Science of Aerosols
« Reply #306 on: May 03, 2024, 07:52:08 PM »
@hausfath
May 1
A lot of folks have been fixated on changes to sulfur in marine fuels of late, but the much bigger climate story here is the nearly 50% decline in overall global emissions of planet-cooling sulfur dioxide since 1980 – much of which has happened in the last 15 years:

May 1, 2024 · 9:50 PM UTC
Patrick Slavenburg - Decision intelligence

I was always puzzled how sulfur-low ship fuel somehow translated into higher (ocean) temperatures.
This sounds as a much more logical - causal - explanation

Zeke Hausfather
Well, sulfur in shipping fuel turns into SO2 and is concentrated over the oceans. Unlike CO2, SO2 is not well mixed in the atmosphere so where it’s emitted matters in terms of cooling impacts.

TrolleyJoe 🍉🕊️
why dont we just start emmitting more sulphur

@hausfath
May 1
Millions of deaths per year from outdoor air pollution? SO2 is really good at forming PM2.5 in the lower atmosphere...

(graphs here)

https://nitter.poast.org/hausfath/status/1785788839996559769#m